5,078 research outputs found
Detection of nanoparticles by means of reflection electron energy loss spectroscopy depth profiling
The various studies of nanoparticles are of great importance because of the wide application of nanotechnology. The shape and structure of the nanoparticles can be determined by transmission electron microscopy (TEM) and their chemistry by electron energy loss spectroscopy. TEM sample preparation is an expensive and difficult procedure, however. Surface sensitive, analytical techniques, such as Auger electron spectroscopy (AES) and x-ray photoelectron spectroscopy (XPS) are well applicable to detect the atoms that make up the nanoparticles, but cannot determine whether particle formation occurred. On the other hand, reflection electron energy loss spectroscopy (REELS) probes the electronic structures of atoms, which are strongly different for the atoms being in solution or in precipitated form. If the particle size is in the nm range, plasmon resonance can be excited in it, which appears as a loss feature in REELS spectrum. Thus, by measuring AES (XPS) spectra parallel with those of REELS, besides the atomic concentrations the presence of the nanoparticles can also be identified. As an example, the appearance of nanoparticles during ion beam induced mixing of C/Si layer will be shown
Nuclear Ground-State Masses and Deformations
We tabulate the atomic mass excesses and nuclear ground-state deformations of
8979 nuclei ranging from O to . The calculations are based on the
finite-range droplet macroscopic model and the folded-Yukawa single-particle
microscopic model. Relative to our 1981 mass table the current results are
obtained with an improved macroscopic model, an improved pairing model with a
new form for the effective-interaction pairing gap, and minimization of the
ground-state energy with respect to additional shape degrees of freedom. The
values of only 9 constants are determined directly from a least-squares
adjustment to the ground-state masses of 1654 nuclei ranging from O to
106 and to 28 fission-barrier heights. The error of the mass model is
0.669~MeV for the entire region of nuclei considered, but is only 0.448~MeV for
the region above .Comment: 50 pages plus 20 PostScript figures and 160-page table obtainable by
anonymous ftp from t2.lanl.gov in directory masses, LA-UR-93-308
Microscopic Enhancement of Heavy-Element Production
Realistic fusion barriers are calculated in a macroscopic-microscopic model
for several soft-fusion heavy-ion reactions leading to heavy and superheavy
elements. The results obtained in such a realistic picture are very different
from those obtained in a purely macroscopic model. For reactions on 208:Pb
targets, shell effects in the entrance channel result in fusion-barrier
energies at the touching point that are only a few MeV higher than the ground
state for compound systems near Z = 110. The entrance-channel fragment-shell
effects remain far inside the touching point, almost to configurations only
slightly more elongated than the ground-state configuration, where the fusion
barrier has risen to about 10 MeV above the ground-state energy. Calculated
single-particle level diagrams show that few level crossings occur until the
peak in the fusion barrier very close to the ground-state shape is reached,
which indicates that dissipation is negligible until very late in the fusion
process. Whereas the fission valley in a macroscopic picture is several tens of
MeV lower in energy than is the fusion valley, we find in the
macroscopic-microscopic picture that the fission valley is only about 5 MeV
lower than the fusion valley for soft-fusion reactions leading to compound
systems near Z = 110. These results show that no significant
``extra-extra-push'' energy is needed to bring the system inside the fission
saddle point and that the typical reaction energies for maximum cross section
in heavy-element synthesis correspond to only a few MeV above the maximum in
the fusion barrier.Comment: 7 pages. LaTeX. Submitted to Zeitschrift fur Physik A. 5 figures not
included here. Complete preprint, including device-independent (dvi),
PostScript, and LaTeX versions of the text, plus PostScript files of the
figures, available at http://t2.lanl.gov/publications/publications.html or at
ftp://t2.lanl.gov/pub/publications/mehe
Influence of the bulk and surface morphology on adhesion of polystyrene-inter-poly-cross-2-ethylhexyl-methacrylate films and particles
The adhesion behavior of semi-interpenetrating polymer networks (semi-IPNs) of linear polystyrene (PS) in crosslinked poly-2-ethylhexylmethacrylate (EHMA) was studied by variation of the bulk and surface morphology, i.e., domain size, continuity, and concentration in the domains. Semi-IPNs were prepared by liquid-liquid demixing upon cooling of a homogeneous solution of PS in methacrylate monomer, followed by gelation of the PS-rich phase and UV polymerization of the methacrylate resin. Welding of films allowed the preparation of larger objects provided that (1) the samples were phase separated to a high degree and contained domains with a high PS concentration (>90%) and (2) polystyrene was present at the interface. For semi-IPN films, a linear dependence of the adhesion strength on the (crack healing time)1/4 was obtained. Based on these considerations, a process was developed to obtain melt-processable semi-IPN particles, by quenching droplets of the polymer solution into a cold liquid. These particles obtained a PS-rich skin layer and showed good adhesion after blending with a thermoplast
TRIDYN_FZR User Manual
The present report contains the User Manual of the FZR version of the dynamic binary-collision computer simulation code TRIDYN. The present version of the code is based on TRIDYN Vs. 4.0 by W.Möller and W.Eckstein, Department of Surface Physics, Max-Planck Institute of Plasma Physics, Boltzmannstraße 2, 85748 Garching, Germany (1989). Modifications, in particular for PC implementation, quasi-dynamic display and the input dialog have been performed at the Institute of Ion Beam Physics and Materials Research by V.Kharlamov, T.Schwieger, M.Posselt, and W.Möller (1995-2001)
Fission-fragment mass distributions from strongly damped shape evolution
Random walks on five-dimensional potential-energy surfaces were recently
found to yield fission-fragment mass distributions that are in remarkable
agreement with experimental data. Within the framework of the Smoluchowski
equation of motion, which is appropriate for highly dissipative evolutions, we
discuss the physical justification for that treatment and investigate the
sensitivity of the resulting mass yields to a variety of model ingredients,
including in particular the dimensionality and discretization of the shape
space and the structure of the dissipation tensor. The mass yields are found to
be relatively robust, suggesting that the simple random walk presents a useful
calculational tool. Quantitatively refined results can be obtained by including
physically plausible forms of the dissipation, which amounts to simulating the
Brownian shape motion in an anisotropic medium.Comment: 14 pages, 11 ps figure
The RF power coupler development programme at LAL-Orsay and DESY-Hamburg for TESLA and the European X-FEL
In the context of a collaboration between LAL (Orsay) and DESY (Hamburg) a programme of development and tests of proto-type power couplers for superconducting cavities is underway in Orsay. Such couplers need to be developed for linear accelerators which require high gradient superconducting cavities, such as the European X-ray Free Electron Laser or the International Linear Collider (ILC) project. We will describe the technical demands which have to be met to build such couplers and will present pro-type designs which are intended to meet these demands, taking the ILC as an example. A description of the infra-structure necessary for the coupler development will also be given along with first high power tests results on a series of power couplers built in industry
Platelet monoamine oxidase activity in alcoholics with and without a family history of alcoholism
A number of studies point at platelet monoamine oxidase (MAO) activity being reduced in alcoholics with a family history of drinking, this being a possible vulnerability marker for alcoholism. To test this hypothesis, we examined a group of recently detoxified alcoholics with high (n = 25) and low genetic loading for alcoholism (n = 28) and a group of healthy controls (n = 21). Clinical assessments were made using the SCID II interview for psychiatric disorders, the Family History Assessment Module and the Semi-Structural Assessment of Genetics in Alcoholism, a questionnaire especially designed for genetic studies. Platelet MAO activity with and without ethanol stimulation and the percentage of MAO activity with ethanol did not differ between groups. The only significant difference was a lower inhibition of MAO activity with ethanol in alcoholics both with and without a family history compared to controls. In patients with antisocial personality traits, platelet MAO activity was also not found to be different from other alcoholics. Our findings question the hypothesis of reduced platelet MAO activity to be a possible vulnerability marker for alcoholism. Copyright (C) 2000 S. Karger AG. Basel
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